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中国边缘海(本文特指渤海、黄海和东海,不包括南海)是陆源和海源有机质的重要碳汇。总有机质指标和生物标志物的结果显示,表层沉积物中陆源有机质高值集中在近岸尤其是河口附近;海源有机质在陆架海盆处有高值,受控于海洋生产力和沉积环境。利用多参数指标对表层沉积物中不同来源和不同年龄有机质的贡献比例估算的结果显示,我国边缘海的有机碳埋藏量约13 Mt/a,占全球边缘海沉积物有机碳埋藏量(~138 Mt/a)的~10%,其中陆源有机质的碳埋藏量(3.9 Mt/a)占全球边缘海沉积物陆源有机质埋藏量的7%。若假定陈化土壤有机质和古老有机质主要是陆源物质,则非现代有机质的碳埋藏量为~6Mt/a,占我国边缘海总有机质碳埋藏量的~46%,与全球边缘海沉积物中陆源有机质的平均比例(44%)相当。这些结果表明我国边缘海在全球海洋碳循环中具有重要地位。本文利用已发表的文献数据,总结和归纳了中国边缘海沉积有机质来源及其碳汇意义。
Abstract:China marginal seas(CMS,including the Bohai Sea,the Yellow Sea,the East China Sea),are a significant sink for both terrestrial organic matter(TOM)and marine OM(MOM).Both the sources and distributions of OM in China marginal seas have been affected by rapid climate changes and anthropogenic activities over the last 60 years.The total organic carbon(TOC)proxies and biomarker results of surface sediments indicated that higher percentage of TOM(%TOM)occurred near coastal regions and especially near river mouths such as the Yellow River Estuary,the old Huanghe Estuary and the Changjiang River Estuary.Higher percentage of MOM values were found in shelf sea basins,controlled by the marine primary production and depositional settings.Quantitative estimates based on both TOC and biomarker proxies with binary or ternary models revealed that total a sequestration of 13Mt/a TOC buried in CMS(~10% of global continental margin sediments)and burial TOM accounted for7%that of global continental margin sediments.If we assumed non-modern OM(including pre-aged and fossil OM)was mainly terrigenous,then the percentage of non-modern OM in CMS was ~46%,comparable to the%TOM(44%)of global continental margin sediments.The preliminary carbon budget in the CMS indicated that it plays an important role in the global marine carbon cycle.This paper sunmaries the sources of sedimentary organic matter in china maginal sea surface sedments and implications of carbon sink using published data.
[1]Burdige D J.Burial of terrestrial organic matter in marine sediments:A re-assessment[J].Global Biogeochemical Cycles,2005,19(4):GB4011.
[2]Galy V,France-Lanord C,Beyssac O,et al.Efficient organic carbon burial in the Bengal fan sustained by the Himalayan erosional system[J].Nature,2007,450(7168):407-410.
[3]Hedges J I,Keil R G.Sedimentary organic matter preservation:an assessment and speculative synthesis[J].Marine Chemistry,1995,49(2):81-115.
[4]Battle M,Bender M,Tans P P,et al.Global carbon sinks and their variability inferred from atmospheric O2andδ13 C[J].Science,2000,287(5462):2467-2470.
[5]Milliman J D,Meade R H.World-wide delivery of river sediment to the oceans[J].The Journal of Geology,1983,91(1):1-21.
[6]李军,胡邦琦,窦衍光,等.中国东部海域泥质沉积区现代沉积速率及其物源控制效应初探[J].地质论评,2012,58(4):745-756.Li Jun,Hu Bangqi,Dou Yanguang,et al.Modern sedimentation rate,budget and supply of the muddy deposits in the East China seas[J].Geological Review,2012,58(4):745-756.
[7]Hu L,Shi X,Bai Y,et al.Recent organic carbon sequestration in the shelf sediments of the Bohai Sea and Yellow Sea,China[J].Journal of Marine Systems,2016,155:50-58.
[8]Deng B,Zhang J,Wu Y.Recent sediment accumulation and carbon burial in the East China Sea[J].Global Biogeochemical Cycles,2006,20(3):GB3014.
[9]Wu Y,Eglinton T,Yang L,et al.Spatial variability in the abundance,composition,and age of organic matter in surficial sediments of the East China Sea[J].Journal of Geophysical Research:Biogeosciences,2013,118(4):1495-1507.
[10]Xing L,Zhang H,Yuan Z,et al.Terrestrial and marine biomarker estimates of organic matter sources and distributions in surface sediments from the East China Sea shelf[J].Continental Shelf Research,2011,31(10):1106-1115.
[11]Blair N E and Aller R C.The fate of terrestrial organic carbon in the marine environment[J].Annual Review of Marine Science,2012,4:401-423.
[12]Drenzek N J,Montlu9on D B,Yunker M B,et al.Constraints on the origin of sedimentary organic carbon in the Beaufort Sea from coupled molecular 13C and 14C measurements[J].Marine Chemistry,2007,103(1):146-162.
[13]Feng X,Benitez-Nelson B C,Montlu9on D B,et al.14C and 13C characteristics of higher plant biomarkers in Washington margin surface sediments[J].Geochimica et Cosmochimica Acta,2013,105:14-30.
[14]Drenzek N J,Hughen K A,Montlu9on D B,et al.A new look at old carbon in active margin sediments[J].Geology,2009,37(3):239-242.
[15]Galy V,Beyssac O,France-Lanord C,et al.Recycling of graphite during Himalayan erosion:A geological stabilization of carbon in the crust[J].Science,2008,322(5903):943-945.
[16]Hedges J I,Keil R G,Benner R.What happens to terrestrial organic matter in the ocean?[J].Organic Geochemistry,1997,27(5-6):195-212.
[17]Xing L,Zhao M,Gao W,et al.Multiple proxy estimates of source and spatial variation in organic matter in surface sediments from the southern Yellow Sea[J].Organic Geochemistry,2014,76:72-81.
[18]Liu D,Li X,Emeis K-C,et al.Distribution and sources of organic matter in surface sediments of Bohai Sea near the Yellow River Estuary,China[J].Estuarine,Coastal and Shelf Science,2015,165:128-136.
[19]Zhu C,Wagner T,Talbot H M,et al.Mechanistic controls on diverse fates of terrestrial organic components in the East China Sea[J].Geochimica et Cosmochimica Acta,2013,117:129-143.
[20]Yao P,Yu Z,Bianchi T S,et al.A multiproxy analysis of sedimentary organic carbon in the Changjiang Estuary and adjacent shelf[J].Journal of Geophysical Research:Biogeosciences,2015,120(7):1407-1429.
[21]Hu L,Shi X,Guo Z,et al.Sources,dispersal and preservation of sedimentary organic matter in the Yellow Sea:The importance of depositional hydrodynamic forcing[J].Marine Geology,2013,335(1):52-63.
[22]Wang X,Ma H,Li R,et al.Seasonal fluxes and source variation of organic carbon transported by two major Chinese Rivers:The Yellow River and Changjiang(Yangtze)River[J].Global Biogeochemical Cycles,2012,26(2):GB2025
[23]Tao S,Eglinton T I,Montlu9on D B,et al.Pre-aged soil organic carbon as a major component of the Yellow River suspended load:Regional significance and global relevance[J].Earth and Planetary Science Letters,2015,414:77-86.
[24]Tao S,Eglinton T I,Montlu9on D B,et al.Diverse origins and pre-depositional histories of organic matter in contemporary Chinese marginal sea sediments[J].Geochimica et Cosmochimica Acta,2016,191:70-88
[25]Bao R,McIntyre C,Zhao M,et al.Widespread dispersal and aging of organic carbon in shallow marginal seas[J].Geology,2016,44(10):791-794
[26]Xing L,Tao S,Zhang H,et al.Distributions and origins of lipid biomarkers in surface sediments from the southern Yellow Sea[J].Applied Geochemistry,2011,26(8):1584-1593.
[27]Eglinton T I,Eglinton G.Molecular proxies for paleoclimatology[J].Earth and Planetary Science Letters,2008,275(1-2):1-16.
[28]Hedges J I,Mann D C.The lignin geochemistry of marine sediments from the southern Washington coast[J].Geochimica et Cosmochimica Acta,1979,43(11):1809-1818.
[29]Hopmans E C,Weijers J W H,SchefuE,et al.A novel proxy for terrestrial organic matter in sediments based on branched and isoprenoid tetraether lipids[J].Earth and Planetary Science Letters,2004,224(1):107-116.
[30]王星辰,邢磊,张海龙,等.北黄海-渤海表层沉积物中浮游植物生物标志物的分布特征及指示意义[J].中国海洋大学学报(自然科学版),2014,44(5):69-73.Wang Xingchen,Xing Lei,Zhang Hailong,et al.Distribution of phytoplantion biomarkers in surface sediments from the north Yellow sea and the Bohai sea and its implication[J].Periodical of Ocean university of China,2014,44(5):69-73.
[31]Hu L,Guo Z,Feng J,et al.Distributions and sources of bulk organic matter and aliphatic hydrocarbons in surface sediments of the Bohai Sea,China[J].Marine Chemistry,2009,113(3):197-211.
[32]Butman D E,Wilson H F,Barnes R T,et al.Increased mobilization of aged carbon to rivers by human disturbance[J].Nature Geoscience,2015,8:112-116.
[33]Galy V,Peucker-Ehrenbrink B,Eglinton T.Global carbon export from the terrestrial biosphere controlled by erosion[J].Nature,2015,521(7551):204-207.
基本信息:
DOI:10.16441/j.cnki.hdxb.20170003
中图分类号:P736.21
引用信息:
[1]赵美训,丁杨,于蒙.中国边缘海沉积有机质来源及其碳汇意义[J],2017,47(09):70-76.DOI:10.16441/j.cnki.hdxb.20170003.
基金信息:
国家重点研发计划项目(2016YFA0601403);; 国家自然科学基金项目(41520104009)资助~~
2017-01-03
2017
2018-03-29
2018
2017-04-07
2