| 386 | 8 | 90 |
| 下载次数 | 被引频次 | 阅读次数 |
对国内外学者近年来在大气干沉降对海域微量金属输入方面的研究工作做了较为系统的综述 :包括样品采集、分析、干沉降通量估算和污染物来源识别。重点讨论了常用分析方法的优缺点以及它们在气溶胶物理、化学性质研究中的应用和已取得的成果 ,旨在为气溶胶分析方法的选择提供参考。
Abstract：The recent researches on the input of trace metal elements to the oceans via atmospheric aerosol dry deposition are reviewed. They include four aspects: aerosol sampling, measurement and analysis, the estimation of dry deposition flux and aerosol source identification. Each analytical technique has its own advantages and disadvantages, which are discussed in detail. To provide reference to the selection of analytical methods, the application and achievement of these techniques in the measurement of physical chemical properties of aerosols are also reported.
[1] 王明星.大气化学.[M]北京:气象出版社,1999:166～244
[2] DuceR A,UnniC K,RayB J,et al.Long-range atmospheric transportof soil dust fromAsia to the tropicalNorthPacific:temporal variability.[J]Science,1980,209:1522～1524
[3] 杨绍晋,杨亦男,陈冰如,等.近中国海域大气微量元素输入量研究.[J]环境化学,1994,13(5):382～387
[4] GolombD,RyanD,EbyN,et al.Atmospheric deposition of toxics onto massachusettsBay-I. metals.[J]AtmosphericEnvironment,1997,31(9):1349～1359
[5] PaodeR D,SofuogluS C,SivadechathepJ,etal.Dry deposition fluxes and mass size distributions ofPb,Cu,andZn measured in southernLakeMichigan duringAEOLOS.[J]EnvironSciTechnol,1998,32(11):1629～1635
[6] McMurryP H.A review of atmospheric aerosol measurements.[J]AtmosphericEnvironment,2000,34:1959～1999
[7] 陈立奇,王志红,杨绪林,等.台湾海峡西部海域大气中金属的特征.金属的浓度和粒度分布.[J]海洋学报,1998,20(6):31～37
[8] KoustenogiiP.Aerosol measurements inSiberia.[J]AtmosphericResearch,1997,44:167～173
[9] KertészZ,Borbély-KissI,RajtaI,et al.Analysis of single aerosol particles collected in urban and caveenvironment by proton microprobe.[J]NuclearInstruments andMetals inPhysicsResearchB,2000,161～163:808～813
[10] 刘平生,胡朝辉,刘世杰,等.近海海洋大气颗粒物中元素浓度及粒径分布研究.[J]环境化学,1994,13(6):498～503
[11] 孙昌年,陈建新,曾宪国,等.利用PIXE技术进行大气气溶胶的元素成分分析.[J]核技术,1989,12(11):673～678
[12] ArtaxoP,CastanhoA D,YamasoeM A,etal.Analysis of atmospheric aerosols byPIXE:the importance ofreal time and complementary measurements.[J]NuclearInstruments andMethods inPhysicsResearchB,1990,150:312～321
[13] 藤恩江,胡 伟,吴国平,等.中国四城市空气中粗细颗粒物元素组成特征.[J]中国环境科学,1999,19(3):238～242
[14] CaffreyP F,OndovJM,ZufallM J,et al.Determination of size-dependent dry particle deposition velocitieswith multiple intrinsic tracers.[J]EnvironSciTechnol,1998,32(11):1615～1622
[15] 余 群,陈立奇,高鹏飞.水和稀酸浸体直接石墨炉原子吸收法测定海洋气溶胶中的微量重金属.[J]海洋学报,1991,13(4):581～587
[16] RidameC,GuieuC,Loy¨ e-PilotM D.Trend in total atmospheric deposition fluxes of aluminium,iron,andtrace metals in the northwesternMediterranean over the past decade(1985～1997).[J]JOfGeophysRes,1999,104(D23):30127～30138
[17] 刘昌岭,张 红,李学刚,等.石墨炉原子吸收法连续测定气溶胶中重金属.[J]理化检验——化学分册,1997,33(8):350～357
[18] 常 辉,杨绍晋,董金泉,等.大气气溶胶中元素种态研究.[J]环境化学,2000,19(6):485～499
[19] GaoY,ArimotoR,DuceR A,etal.Inputof atmospheric traceelementsand mineralmatterto theYellowSeaduring the spring of a low-dustyear.[J]JOfGeophysRes,1992,97(D4):3767～3777
[20] 林学辉,刘昌岭,张 红.等离子体发射光谱法同时测定大气气溶胶中多种金属元素.[J]岩矿测试,1998,17(2):143～146
[21] PécheyranC,LalèreB,DonardO F X.Volatile metal and metalloid species(Pb,Hg,Se) in aEuropean urbanatmosphere(Bordeaux,France).[J]EnvironSciTechnol,2000,34(1):27～32
[22] ShahinU,YiS M,PaodeR D,et al.Long-term elemental dry deposition fluxes measured aroundLakeMichigan with an automated dry deposition sampler.[J]EnvironSciTechnol,2000,34(10):1887～1892
[23] FlorenceT M.He speciation of trace elementin water.[J]Talanta,1982,29(5):345～364
[24] 蔡 卓,肖少荣,郑海林.元素形态分析.[J]广西大学学报(自然科学版),1996,21(3):242～246
[25] KasparianJ,FrejafonE,RambaldiP,etal.Characterization of urban aerosols usingSEM-Microscopy,x-rayanalysis and lidar measurements.[J]AtmosphericEnvironment,1998,32(17):2957～2967
[26] 许 黎,樊小标,石广玉,等.对流层平流层气溶胶粒子的形态和化学组成.[J]气象学报,1998,56(5):551～559
[27] 张代洲,赵春生,秦 瑜.沙尘粒子的成分和形态分析.[J]环境科学学报,1998,18(5):449～456
[28] 汪安璞,杨淑兰,沙 因.北京大气气溶胶单个颗粒的化学表征.[J]环境化学,1996,15(6):488～495
[29] 沙 因,石 践,章佩群,等.用核子微探针进行单个大气颗粒物的分析.[J]环境化学,1995,14(6):518～523
[30] WangJ,GuoP,LiX,et al.Source identification of lead pollution in the atmosphere ofShanghaiCity byanalyzing single aerosol particles.[J]EnvironSciTechno,2000,34(10):1900～1905
[31] HinzK P,KaufmannR,SpenglerB.On-line measurement and characterization of single particles using lasermass spectrometry and multivariate data analysis.[J]JAerosolSci,1996,27:3171～3172
[32] 高 原,DuceR A.沿海海-气界面的化学物质交换.[J]地球科学进展,1997,12(6):553～563
[33] GESAMP(Group ofExperts onScientificAspects ofMarinePollution)WorkingGroup14.The atmosphericInputofTraceSpecies to theWorldOcean.[R]RepStud38.Geneva:WorldMeteorolUrgan,1989:106
[34] WilliamsR W.A model for the dry deposition of particles to natural water surface.[J]AtmosphericEnvironment,1982,16(8):1933～1938
[35] 刘 毅,周明煜.中国东部海域大气气溶胶入海通量的研究.[J]海洋学报,1999,21(5):38～45
[36] 王喜全.适用于大中尺度污染物输送模式的粒子干沉降参数化方案.[J]气候与环境研究,1998,3(2):125～133
[37] 张 强,胡隐樵,黄世鸿.估算大气边界层内气溶胶中干沉降速度和浓度垂直分布方法.[J]甘肃科学学报,1995,7(4):50～57
[38] ZhangL,GongS,PadroJ,etal.A size-segregated particle dry deposition scheme for an atmospheric aerosolmodule.[J]AtmosphericEnvironment,2001,35:549～560
[39] 祁士华,傅家谟,盛国英,等.大气气溶胶物质来源研究进展.[J]环境科学进展,1999,7(6):26～30
[40] 陈立奇,王志红,杨绪林,等.台湾海峡西部海域大气中金属的特征.大气颗粒金属的来源和入海通量.[J]海洋学报,1999,21(1):23～30
[41] ArnoldE,MerrillJ,LeinenM,et al.The effect of source area and atmospheric transport on mineral aerosolcollected over theNorthPacificOcean.[J]Global andPlnetaryChange,1998,18:151～159
[42] 全 浩.关于中国西部地区沙尘暴及其黄沙气溶胶高空传输路线的探讨.[J]环境科学,1993,14(5):60～64
[43] 刘 毅,周明煜.北京及近中国海春季气溶胶浓度变化规律的研究.[J]环境科学学报,1999,19(6):642～647
[44] 庄国顺,郭敬华,袁 蕙,等.2000年我国沙尘暴的组成、来源、粒径分布及其对全球环境的影响.[J]科学通报,2001,46(3):191～197
基本信息:
DOI：10.16441/j.cnki.hdxb.2002.03.020
中图分类号:P734
引用信息:
[1]张曼平,祁建华,冯丽娟,李先国.大气气溶胶干沉降对海域微量金属输入的研究现状[J].青岛海洋大学学报(自然科学版),2002(03):449-455.DOI:10.16441/j.cnki.hdxb.2002.03.020.
基金信息:
国家自然科学基金项目 ( 4 9976 0 2 0 )
2002-06-30
2002-06-30