北黄海夏季pCO2分布及海-气CO2通量Surface pCO2 and Air-Sea CO2 Flux in the Northern Yellow Sea During Summer
薛亮,张龙军
摘要(Abstract):
基于在2006年夏季北黄海收集的的高分辨率的表层CO2分压(pCO2)数据,结合水文和生物地球化学同步观测参数,探讨了夏季北黄海pCO2空间分布的控制因素。结果表明,夏季北黄海与大多数中低纬度陆架海类似,由于水温较高,表层pCO2较高(平均值为(463±41)μatm),整个海域相对大气CO2过饱和。表层pCO2分布具有明显的区域差异,辽南和鲁北近岸海域pCO2明显高于中部区域,辽南近岸的高pCO2主要与河流输入和水产养殖引起的生物好氧呼吸有关,而鲁北沿岸的高pCO2主要与烟台近岸的底层冷水涌升及由混合引起的高碳酸盐含量的黄河泥沙的再悬浮有关;在海区中部大部分水域,pCO2与温度之间有较好的相关性,说明温度是这一区域pCO2分布较为重要的控制因子。另外,采用Wannikhof的海-气气体交换系数估计了北黄海夏季海-气CO2通量,结果表明整个北黄海是大气CO2的源,平均释放速率为(4.00±0.57)mmol.m-2.d-1,高于南黄海夏季海-气CO2通量。
关键词(KeyWords): 表层pCO2;控制因素;海-气CO2通量;北黄海
基金项目(Foundation): 国家908专项(908-01-ST02)资助
作者(Author): 薛亮,张龙军
DOI: 10.16441/j.cnki.hdxb.2011.12.004
参考文献(References):
- [1]Tsunogai S,Watanabe S,Sato T.Is there a“continental shelfpump”for the absorption of atmospheric CO2?[J].Tellus B,1999,51(3):701-712.
- [2]Thomas H,Bozec Y,Elkalay K,et al.Controls of the surfacewater partial pressure of CO2in the North Sea[J].Biogeoscienc-es,2005,2:323-334.
- [3]Thomas H,Bozec Y,Elkalay K,et al.Enhanced open ocean stor-age of CO2from shelf sea pumping[J].Science,2004,304(5673):1005-1008.
- [4]Jiang L-Q,Cai W-J,Wanninkhof R,et al.Air-sea CO2fluxes onthe U.S.South Atlantic Bight:Spatial and seasonal variability[J].J Geophys Res,2008,113 C07019,doi:10.1029/2007JC004366.
- [5]Cai W-J,Wang Z A,Wang Y.The role of marsh-dominated het-erotrophic continental margins in transport of CO2between the at-mosphere,the land-sea interface and the ocean[J].Geophys ResLett,2003,30(16):18-49.doi:10.1029/2003GL017633.
- [6]Ducklow H W,Mccallister S L.The biogeochemistry of carbon di-oxide in the coastal oceans[M].∥Robinson A R,Mccarthy J,Rothschild B J,eds.The Sea.[s.l.]:The Global Coastal Ocean:Multiscale Interdisciplinary Processes,2005:269-315.
- [7]Gattuso J P,Frankignoulle M,Wollast R.Carbon and carbonatemetabolism in coastal aquatic ecosystems[J].Annual Review ofEcology and Systematics,1998,29(1):405-434.
- [8]Fennel K.The role of continental shelves in nitrogen and carboncycling:Northwestern North Atlantic case study[J].Ocean Sci,2010,6(2):539-548.
- [9]Degrandpre M D,Olbu G J,Beatty C M,et al.Air-sea CO2fluxeson the US Middle Atlantic Bight[J].Deep Sea Research Part II,2002,49(20):4355-4367.
- [10]Xue L,Zhang L,Cai W-J,et al.Air-sea CO2fluxes in the south-ern Yellow Sea:an examination of the continental shelf pump hy-pothesis[J].Continental Shelf Research,doi:10.1016/j.csr.2011.09.002.
- [11]Cai W-J,Dai M.Comment on“Enhanced open ocean storage ofCO2from shelf sea pumping”[J].Science,2004,306(5701):1477c.
- [12]Cai W J,Dai M,Wang Y.Air-sea exchange of carbon dioxide inocean margins:A province-based synthesis[J].Geophys ResLett,2006,33,L12603,doi:10.1029/2006GL026219.
- [13]Borges A.Do we have enough pieces of the jigsaw to integrateCO2fluxes in the coastal ocean?[J].2005,28(1):3-27.
- [14]Borges A V,Delille B,Frankignoulle M.Budgeting sinks andsources of CO2in the coastal ocean:Diversity of ecosystemscounts[J].Geophys Res Lett,2005,32,L14601,doi:10.1029/2005GL023053.
- [15]Chen C T A,Borges A V.Reconciling opposing views on carboncycling in the coastal ocean:Continental shelves as sinks andnear-shore ecosystems as sources of atmospheric CO2[J].DeepSea Research Part II,2009,56(8-10):578-590.
- [16]Liu K,Atkinson L,Quin珘ones R,et al.Carbon and nutrient flu-xes in continental margins:A Global Synthesis[M].Verlag Ber-lin Heidelberg:Springer,2010.
- [17]Takahashi T,Sutherland S C,Wanninkhof R,et al.Climatolog-ical mean and decadal change in surface ocean pCO2,and net sea-air CO2flux over the global oceans[J].Deep Sea Research PartII,2009,56(8-10):554-577.
- [18]Doney S C,Tilbrook B,Roy S,et al.Surface-ocean CO2varia-bility and vulnerability[J].Deep Sea Research Part II,2009,56(8-10):504-511.
- [19]Cai W J.Estuarine and coastal ocean carbon paradox:CO2sinksor sites of terrestrial carbon incineration[J].Annual Review ofMarine Science,2011,3:123-145.
- [20]Zhang L,Xue L,Song M,et al.Distribution of the surface par-tial pressure of CO2in the southern Yellow Sea and its controls[J].Continental Shelf Research,2010,30:293-304.
- [21]张龙军,郭朝,薛亮.秋季北黄海表层海水CO2分压分布及其影响因素探讨[J].中国海洋大学学报:自然科学版,2009,39(4):587-591.
- [22]孙同美,张龙军,薛亮.春季北黄海表层海水CO2分压分布及其影响因素探讨[J].中国海洋大学学报:自然科学版,2009,39(sup.):171-176.
- [23]张龙军,王婧婧,张云,等.冬季北黄海表层海水pCO2分布及其影响因素探讨[J].中国海洋大学学报:自然科学版,2008,38(6):955-960.
- [24]Su J.Chapter 16Circulation dynamics of the China Seas north of18°N coastal segment[M].∥Robinson A R,Brink K H,TheSea.[s.l.]:John Wiley&Sons,Inc,1998:483-505.
- [25]鲍献文,李娜,姚志刚,等.北黄海温盐分布季节变化特征分析[J].中国海洋大学学报:自然科学版,2009,39(4):553-562.
- [26]Wu Y,Zhang J.Carbon isotope geochemistry in the Yalujiangestuary[J].Science in China(Series B),2001,44(sup):173-176.
- [27]Wang Z A,Cai W J.Carbon dioxide degassing and inorganic car-bon export from a marsh-dominated estuary(the Duplin River):A marsh CO2pump[J].Limnology and Oceanography,2004,49(2):341-354.
- [28]ftp://ftp.cmdl.noaa.gov/ccg/CO2/flask/month/.
- [29]李风岐,苏育嵩.海洋水团分析[M].青岛:青岛海洋大学出版社,1999.
- [30]张龙军,张云.夏季渤海表层海水pCO2分布特征[J].中国海洋大学学报:自然科学版,2008,38(4):635-639.
- [31]王晓亮,张龙军,苏征,等.黄河口总碱度保守与非保守行为探讨[J].中国海洋大学学报:自然科学版,2005,35(6):1063-1067.
- [32]王年斌,马志强,薛克,等.黄海北部河口海域无机氮含量的分布动态与环境质量评价[J].大连水产学院学报,2003,18(004):282-286.
- [33]高爽,李正炎.北黄海夏、冬季叶绿素和初级生产力的空间分布和季节变化特征[J].中国海洋大学学报:自然科学版,2009,39(4):604-610.
- [34]Schiettecatte L S,Thomas H,Vieira Borges A,et al.Normal-ized total alkalinity as a tracer of the surface seawater masses ofthe North Sea[Z].France:Nice,2003:1.
- [35]Millero F J.The marine inorganic carbon cycle[J].Chemical Re-views,2007,107(2):308-341.
- [36]Takahashi T,Olafsson J,Goddard J G,et al.Seasonal variationof CO2and nutrients in the high-latitude surface oceans:a com-parative study[J].Global Biogeochem Cycles,1993,7(4):843-878.
- [37]Gieskes J M.Effect of temperature on the pH of seawater[J].Limnology and Oceanography,1969,14(5):679-685.
- [38]于非,张志欣,刁新源,等.黄海冷水团演变过程及其与邻近水团关系的分析[J].海洋学报,2006,28(5):26-34.
- [39]Lohrenz S E,Cai W,Chen F,et al.Seasonal variability in air-sea fluxes of CO2in a river-influenced coastal margin[J].J Geo-phys Res,2010,115,C10034,doi:10.1029/2009JC005608.
- [40]李岩,张龙军,苏征,等.长江口淡水端淡、盐水混合表层pCO2的急剧变化及其影响机制[J].中国海洋大学学报:自然科学版,2006,36(2):295-298.
- [41]Jiang L Q,Cai W J,Wang Y.A comparative study of carbon di-oxide degassing in river-and marine-dominated estuaries[J].Limnology and Ocenography,2008,53(6):2603-2615.
- [42]Krasakopoulou E,Rapsomanikis S,Papadopoulos A,et al.Par-tial pressure and air-sea CO2flux in the Aegean Sea during Febru-ary 2006[J].Continental Shelf Research,2009,29(11/12):1477-1488.
- [43]史华明,王丽莎,石晓勇.北黄海溶解无机氮组成,分布及季节变化特征[J].中国海洋大学学报:自然科学版,2009,39(Sup.):207-211.
- [44]鲍献文,李真,王勇智,等.冬、夏季北黄海悬浮物分布特征[J].泥沙研究,2010,2:48-56.
- [45]王桂芝,高抒.黄渤海水体交换,悬沙特征及其对渤海海峡沉积的影响[J].海洋通报,2002,21(001):43-48.
- [46]Weiss R F.Carbon dioxide in water and seawater:the solubilityof a non-ideal gas[J].Marine Chemistry,1974,2:203-215.
- [47]Wanninkhof R.Relationship Between Wind Speed and Gas Ex-change Over the Ocean[J].J Geophys Res,1992,97(C5):7373-7382.
- [48]http://las.pfeg.noaa.gov/oceanWatch/oceanwatch.php.
文章评论(Comment):
|
||||||||||||||||||
|
||||||||||||||||||